The Adjustment Bureau
Matt Damon and Emily Blunt shot scenes in Fort Tryon Park in 2009 for this sci-fi romance.
Fort Tryon Park (exact spots not specified in sources)

DNAinfo reported in March 2011 that the stars shot scenes in Fort Tryon Park in 2009, and that the park’s New Leaf Cafe was offering a free glass of wine for movie-ticket stubs that month. The report does not say which scenes or where in the park, so the local tie is documented but unspecific.